Directional dichroism in the paramagnetic state of multiferroics: A case study of infrared light absorption in Sr2CoSi2 O7 at high temperatures

J. Viirok, U. Nagel, T. Rõõm, D. G. Farkas, P. Balla, D. Szaller, V. Kocsis, Y. Tokunaga, Y. Taguchi, Y. Tokura, B. Bernáth, D. L. Kamenskyi, I. Kézsmárki, S. Bordács, K. Penc

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2 Citations (Scopus)

Abstract

The coexisting magnetic and ferroelectric orders in multiferroic materials give rise to a handful of novel magnetoelectric phenomena, such as the absorption difference for the opposite propagation directions of light called the nonreciprocal directional dichroism (NDD). Usually, these effects are restricted to low temperature, where the multiferroic phase develops. In this paper, we report the observation of NDD in the paramagnetic phase of Sr2CoSi2O7 up to temperatures more than 10 times higher than its Néel temperature (7 K) and in fields up to 30 T. The magnetically induced polarization and NDD in the disordered paramagnetic phase is readily explained by the single-ion spin-dependent hybridization mechanism, which does not necessitate correlation effects between magnetic ions. The Sr2CoSi2O7 provides an ideal system for a theoretical case study, demonstrating the concept of magnetoelectric spin excitations in a paramagnet via analytical as well as numerical approaches. We applied exact diagonalization of a spin cluster to map out the temperature and field dependence of the spin excitations, as well as symmetry arguments of the single ion and lattice problem to get the spectrum and selection rules.

Original languageEnglish
Article number014410
JournalPhysical Review B
Volume99
Issue number1
DOIs
Publication statusPublished - jan. 9 2019

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ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Condensed Matter Physics

Cite this

Viirok, J., Nagel, U., Rõõm, T., Farkas, D. G., Balla, P., Szaller, D., Kocsis, V., Tokunaga, Y., Taguchi, Y., Tokura, Y., Bernáth, B., Kamenskyi, D. L., Kézsmárki, I., Bordács, S., & Penc, K. (2019). Directional dichroism in the paramagnetic state of multiferroics: A case study of infrared light absorption in Sr2CoSi2 O7 at high temperatures. Physical Review B, 99(1), [014410]. https://doi.org/10.1103/PhysRevB.99.014410