On the limitations introduced by energy spread in elastic recoil detection analysis

Research output: Contribution to journalArticle

10 Citations (Scopus)

Abstract

Improvements in experimental techniques have led to monolayer depth resolution in heavy ion elastic recoil detection analysis (HI-ERDA). Evaluation of the spectra, however, is not trivial. The spectra, using even the best experimental set-up, are subject to finite energy resolution of both extrinsic and intrinsic origin. A proper account for energy spread is necessary to extract the correct depth profile from the measured spectra. With calculation of the correct energy (or depth) resolution of a given method, one can decide in advance whether or not the method will resolve details of interest in the depth profile. To achieve the best depth resolution, it is also possible to find optimum parameters for the experiments. The limitations introduced by the energy spread effects are discussed. An example for simulation is shown for high energy resolution HI-ERDA measurements. Satisfactory agreement between the simulated and the measured HI-ERDA spectra taken by 60 MeV 127I23+ ions on highly oriented pyrolythic graphite (HOPG) sample is found, in spite of the non-equilibrium charge state of the recoils and the difference in the stopping powers caused by the given charge state of the incident ion and the recoil, which are not taken into account. To achieve more precise data evaluation these effects should be included in simulation codes, or all the subspectra corresponding to different recoils charge states should be measured and summed.

Original languageEnglish
Pages (from-to)25-33
Number of pages9
JournalNuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms
Volume183
Issue number1-2
DOIs
Publication statusPublished - Jul 2001

Fingerprint

Heavy Ions
Heavy ions
heavy ions
Ions
Graphite
Spectrum analysis
energy
Monolayers
evaluation
stopping power
profiles
spectrum analysis
ions
simulation
graphite
Experiments

Keywords

  • Depth resolution
  • Elastic recoil detection analysis
  • Energy resolution
  • Simulation

ASJC Scopus subject areas

  • Surfaces, Coatings and Films
  • Instrumentation
  • Surfaces and Interfaces

Cite this

@article{88e6b15de6da4b0d982c0d30e3abf7ac,
title = "On the limitations introduced by energy spread in elastic recoil detection analysis",
abstract = "Improvements in experimental techniques have led to monolayer depth resolution in heavy ion elastic recoil detection analysis (HI-ERDA). Evaluation of the spectra, however, is not trivial. The spectra, using even the best experimental set-up, are subject to finite energy resolution of both extrinsic and intrinsic origin. A proper account for energy spread is necessary to extract the correct depth profile from the measured spectra. With calculation of the correct energy (or depth) resolution of a given method, one can decide in advance whether or not the method will resolve details of interest in the depth profile. To achieve the best depth resolution, it is also possible to find optimum parameters for the experiments. The limitations introduced by the energy spread effects are discussed. An example for simulation is shown for high energy resolution HI-ERDA measurements. Satisfactory agreement between the simulated and the measured HI-ERDA spectra taken by 60 MeV 127I23+ ions on highly oriented pyrolythic graphite (HOPG) sample is found, in spite of the non-equilibrium charge state of the recoils and the difference in the stopping powers caused by the given charge state of the incident ion and the recoil, which are not taken into account. To achieve more precise data evaluation these effects should be included in simulation codes, or all the subspectra corresponding to different recoils charge states should be measured and summed.",
keywords = "Depth resolution, Elastic recoil detection analysis, Energy resolution, Simulation",
author = "E. Szil{\'a}gyi",
year = "2001",
month = "7",
doi = "10.1016/S0168-583X(01)00457-8",
language = "English",
volume = "183",
pages = "25--33",
journal = "Nuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms",
issn = "0168-583X",
publisher = "Elsevier",
number = "1-2",

}

TY - JOUR

T1 - On the limitations introduced by energy spread in elastic recoil detection analysis

AU - Szilágyi, E.

PY - 2001/7

Y1 - 2001/7

N2 - Improvements in experimental techniques have led to monolayer depth resolution in heavy ion elastic recoil detection analysis (HI-ERDA). Evaluation of the spectra, however, is not trivial. The spectra, using even the best experimental set-up, are subject to finite energy resolution of both extrinsic and intrinsic origin. A proper account for energy spread is necessary to extract the correct depth profile from the measured spectra. With calculation of the correct energy (or depth) resolution of a given method, one can decide in advance whether or not the method will resolve details of interest in the depth profile. To achieve the best depth resolution, it is also possible to find optimum parameters for the experiments. The limitations introduced by the energy spread effects are discussed. An example for simulation is shown for high energy resolution HI-ERDA measurements. Satisfactory agreement between the simulated and the measured HI-ERDA spectra taken by 60 MeV 127I23+ ions on highly oriented pyrolythic graphite (HOPG) sample is found, in spite of the non-equilibrium charge state of the recoils and the difference in the stopping powers caused by the given charge state of the incident ion and the recoil, which are not taken into account. To achieve more precise data evaluation these effects should be included in simulation codes, or all the subspectra corresponding to different recoils charge states should be measured and summed.

AB - Improvements in experimental techniques have led to monolayer depth resolution in heavy ion elastic recoil detection analysis (HI-ERDA). Evaluation of the spectra, however, is not trivial. The spectra, using even the best experimental set-up, are subject to finite energy resolution of both extrinsic and intrinsic origin. A proper account for energy spread is necessary to extract the correct depth profile from the measured spectra. With calculation of the correct energy (or depth) resolution of a given method, one can decide in advance whether or not the method will resolve details of interest in the depth profile. To achieve the best depth resolution, it is also possible to find optimum parameters for the experiments. The limitations introduced by the energy spread effects are discussed. An example for simulation is shown for high energy resolution HI-ERDA measurements. Satisfactory agreement between the simulated and the measured HI-ERDA spectra taken by 60 MeV 127I23+ ions on highly oriented pyrolythic graphite (HOPG) sample is found, in spite of the non-equilibrium charge state of the recoils and the difference in the stopping powers caused by the given charge state of the incident ion and the recoil, which are not taken into account. To achieve more precise data evaluation these effects should be included in simulation codes, or all the subspectra corresponding to different recoils charge states should be measured and summed.

KW - Depth resolution

KW - Elastic recoil detection analysis

KW - Energy resolution

KW - Simulation

UR - http://www.scopus.com/inward/record.url?scp=0035398644&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=0035398644&partnerID=8YFLogxK

U2 - 10.1016/S0168-583X(01)00457-8

DO - 10.1016/S0168-583X(01)00457-8

M3 - Article

AN - SCOPUS:0035398644

VL - 183

SP - 25

EP - 33

JO - Nuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms

JF - Nuclear Instruments and Methods in Physics Research, Section B: Beam Interactions with Materials and Atoms

SN - 0168-583X

IS - 1-2

ER -